View Starred / Favourite Contacts
Proton Mail for Web should allow marking individual contacts as "Starred" or "Favourite".
Coinciding with that, the Contacts pane should have a "Starred" or "Favourites" tab in addition to "Contacts" and "Groups".
Although this is not a critical feature, there are already at least two good reasons for it:
All of the extra encrypted fields in Contacts makes Proton Mail a good place not just to store your e-mail contacts, but your entire address book, including phone numbers, mailing addresses, birthdates (etc). However, this leads to the addition of many seldom-used entries that one doesn't necessarily need or want to see on the main list.
If "Automatically Save Contacts" is turned ON (which seems to be the default), the "Starred / Favourites" view will remain clean. I personally turned this feature OFF because I didn't want additional automatically-added Contacts entries clogging up my address book, but would have left it enabled if the feature I'm proposing existed.
In the Proton Mail for ANDROID app: if the intention is to continue showing all contacts and groups in a single consolidated list, the starred / favourite ones could simply sort to the top.